文章摘要
Research Progress of Dynamically Crosslinked Silicone Elastomers
Received:April 18, 2024  Revised:April 18, 2024
DOI:10.12136/j.issn.1000-890X.2025.09.0712
Key Words: silicone elastomer;polysiloxane;dynamic crosslinking;non-covalent bond;covalent bond;self-healing
Author NameAffiliationE-mail
YUE Xuejun China Academy of Engineering Physics yuexuejun2022@163.com 
LU Ai China Academy of Engineering Physics  
KANG Ming Southwest University of Science and Technology  
YU Fengmei* China Academy of Engineering Physics yufengmei_icm@163.com 
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Abstract:
      Research progress of silicone elastomers based on dynamic non-covalent bond crosslinking,dynamic covalent bond crosslinking and multiple dynamic bond synergistic effect was reviewed,and the development prospect of dynamically crosslinked silicone elastomers was envisioned.By introducing multiple dynamic crosslinking bonds into the crosslinked network of silicone(polysiloxane),the good physicochemical properties of silicone elastomer were retained,while the novel self-healing pathways and better reprocessability were provided.The synergistic interaction between dynamic covalent bond and dynamic non-covalent bond was recognized as an effective way for achieving excellent mechanical properties and good dynamic behavior of silicone elastomer.The development of dynamically crosslinked silicone elastomers was regarded as a new direction for their high value application and environmentally friendly recycling in intelligent coatings,sensors and flexible electronic devices.
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